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- W2032244571 abstract "The presence of a cyclopentadienyl ligand brings about a complete shift of regioselectivity in the Fe+-mediated dehydrogenation of 1,8-diphenyloctane (1). While “bare” Fe+, due to the formation of an intramolecular sandwich-like complex, activates the internal C-4/C-5 positions of the alkyl chain, this chelate effect is no longer operative in the gas-phase chemistry of Fe(C5H5)+ with 1. Labeling experiments demonstrate that the C-1/C-2 and (to a minor extent) the C-2/C-3 methylene groups are activated, and a possible origin of this remarkable ligand effect is discussed." @default.
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- W2032244571 date "1995-06-01" @default.
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- W2032244571 title "Ligand-Induced Directionality Shift in the Fe+-Mediated Dehydrogenation of 1,8-Diphenyloctane" @default.
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- W2032244571 doi "https://doi.org/10.1002/cber.19951280620" @default.
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