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- W2032343692 abstract "The extension of model Hamiltonian of Kornyshev et al. [Electrochim. Acta 42 (1997) 849] is suggested, and a modified analytical expression for the static nonlocal dielectric function ε(k) of a polar liquid with due account of the ovescreening effect is obtained. The goal is to correct the too small values of some of the fitted correlation lengths presented in the former work. The extension consists in the introduction of a nonlocality into the coupling of one of the polarization modes of a liquid to the scalar field and results in the appearance of a new fitting parameter. The new analytical expression for ε(k) almost retains the form suggested by Kornyshev et al. However, it is shown that the new expression permits to bring the values of fitted parameters into a range where they can be interpreted more realistically. Using the results of computer simulations for ε(k), a number of parameterizations of ε(k) for water, acetonitrile, and dimethyl is obtained and presented." @default.
- W2032343692 created "2016-06-24" @default.
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- W2032343692 date "2004-01-01" @default.
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- W2032343692 title "The analytical expression for the static nonlocal dielectric function of a polar liquid with due account of the overscreening effect" @default.
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- W2032343692 doi "https://doi.org/10.1016/j.electacta.2003.07.002" @default.
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