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• W2032603915 endingPage "1348" @default.
• W2032603915 startingPage "1343" @default.
• W2032603915 abstract "Poly(N-isopropylacrylamide), NIPA, thermoresponsive hydrogels with well-defined concentrations of an electroactive probe, 1,1'-ferrocenedimethanol, Fc(MeOH)2, were prepared. The discontinuous reversible volume phase transition of such gels occurs at 32 +/- 1 degrees C and results in a release of approximately 93% of the solution from the polymeric network. Transport of Fc(MeOH)2 in both swollen and collapsed gels was studied using steady-state voltammetry and chronoamperometry at platinum microelectrodes. The diffusion coefficient of Fc(MeOH)2 in collapsed gels was approximately 2 orders of magnitude smaller than that in swollen gels. UV/vis spectroscopic studies showed that for 3.0% NIPA gel, the concentration of Fc(MeOH)2 in the collapsed phase was approximately 6 times higher than that in released solution and 4.5 times higher than in the original swollen gel." @default.
• W2032603915 created "2016-06-24" @default.
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• W2032603915 date "2002-02-09" @default.
• W2032603915 modified "2023-10-14" @default.
• W2032603915 title "Diffusion and Concentration of Molecular Probes in Thermoresponsive Poly(<i>N</i>-isopropylacrylamide) Hydrogels: Effect of the Volume Phase Transition" @default.
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• W2032603915 doi "https://doi.org/10.1021/ac0107857" @default.
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