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• W2032708682 abstract "Abstract Polarized reflectivity spectra of CaMoO 4 and CaWO 4 single crystals have been measured up to 30 eV by using synchrotron radiation as a light source. The optical constants for a ‐ and c ‐axes are derived from the reflectivity spectra by a Kramers–Kronig analysis. A clear correspondence is found in the main structures of the optical spectra between molybdate and tungstate. It is revealed that the lowest bands peaking at 5.0 eV in CaMoO 4 and at 6.0 eV in CaWO 4 consisit of some fine structures with distinct dichroism. They are attributed to the joint density‐of‐states; in other words, no structures indicative of exciton transition are found at the fundamental absorption edge. From the comparison of the spectral profiles in CaMoO 4 and CaWO 4 , the structures below 10 eV are ascribed to the transitions from the O 2p valence band to the conduction band mainly made of Mo 4d (W 5d) states, while those above 10 eV are assigned to the transitions to the Ca conduction band. The polarization dependence of the structures below 10 eV is explained well in terms of the intramolecular transition in an oxyanion complex in the scheelite crystal. The energy band structure of CaWO 4 is discussed taking into account of the previous results such as the thermostimulated luminescence and the two‐photon excitation. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)" @default.
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• W2032708682 date "2006-05-02" @default.
• W2032708682 modified "2023-10-09" @default.
• W2032708682 title "Comparative study of optical spectra and electronic structures of CaMoO4 and CaWO4 crystals" @default.
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• W2032708682 doi "https://doi.org/10.1002/pssb.200541468" @default.
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