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- W2032796854 abstract "Measurements of ionic clustering equilibria in a high-pressure mass spectrometer source are subject to a systematic error arising from in-flight evaporation. Recent advances in unimolecular rate theory permit a general analysis of this problem. The information necessary for its solution is extracted from evaporation measurements made in other contexts. We consolidate this information in a “best value” for the Gspann parameter which we report as γ = 23.5 (± 1.5). We then find that in typical experimental conditions evaporation is indeed important. Nevertheless, in measurements of an equilibrium constant offsetting errors will ameliorate the severity of this artifact." @default.
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- W2032796854 date "1990-10-01" @default.
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- W2032796854 title "Evaporative corrections to high-pressure ionic clustering data" @default.
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- W2032796854 doi "https://doi.org/10.1016/0168-1176(90)85088-j" @default.
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