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- W2032874530 abstract "Time-dependent density-functional-theory (TDDFT) methods are used to calculate the orientational dependence of ionization and molecular high-order harmonic generation (MHOHG) in the CO${}_{2}$ molecule as a function of laser intensity ${I}_{0}ensuremath{geqslant}{10}^{14}$ W$/$cm${}^{2}$ for few-cycle 800 nm laser pulses. A time-series analysis is used to confirm the recollision model in MHOHG for different density potentials. It is found that at intensities ${I}_{0}>3.5ifmmodetimeselsetexttimesfi{}{10}^{14}$ W$/$cm${}^{2}$, lower highest occupied molecular orbitals (HOMO's) contribute significantly to ionization and to the MHOHG process. This is due to the symmetry of these orbitals. Even though such lower orbitals have higher ionization potentials (IP), ionization and MHOHG processes occur when orbital densities are maximum with laser polarization direction." @default.
- W2032874530 created "2016-06-24" @default.
- W2032874530 creator A5007962222 @default.
- W2032874530 creator A5075008446 @default.
- W2032874530 date "2010-02-16" @default.
- W2032874530 modified "2023-09-30" @default.
- W2032874530 title "Nonlinear time-dependent density-functional-theory study of ionization and harmonic generation in CO<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow /><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>by ultrashort intense laser pulses: Orientational effects" @default.
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- W2032874530 doi "https://doi.org/10.1103/physreva.81.023411" @default.
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