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- W2032912792 abstract "Autoionizing resonance of acetylene is studied by photoelectron spectroscopy using synchrotron radiation. Pronounced vibrational excitation in the C–H stretching mode ν1 is observed in the (1πu)−1X̃ 2Πu band of C2H+2 at a restricted photon energy range from 12.8 to 14.1 eV. It is concluded that the 3σg→3σu autoionizing transition at ∼13.3 eV gives rise to an anomalously broad maximum in the (1πu)−1 photoionization cross section curve. The strong ν1 excitation is explained as that the equilibrium C–H bond length differs from the neutral and ionic ground states to the (3σg)−1(3σu)1 resonance state. Constant ionic state spectra for the v1=3 and 4 levels of the X̃ 2Πu state measured over the same energy region show fine structures with regular spacings corresponding to the vibrational levels of the (3σg)−1(3σu)1 state." @default.
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- W2032912792 date "1995-04-01" @default.
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- W2032912792 title "Autoionizing resonance in photoionization from the 1π<i>u</i> level of acetylene" @default.
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- W2032912792 doi "https://doi.org/10.1063/1.469254" @default.
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