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- W2032982373 abstract "The chemical behavior of 144Pr as a result of the β−-decay of the 144Ce(III)-diethylenetriaminepentaacetate (144Ce(III)-DTPA) complex was investigated in detail on the basis of the substitution reaction mechanism. The experimental results, represented in terms of the yield of the 144Pr(III)-DTPA complex, were explained quantitatively by the application of Bateman’s equation. An increase in the nuclear charge in the β-decay of the 144Ce(III)-DTPA complex may result in the formation of 144Pr(IV)-DTPA, which would then be reduced to an intermediate complex of 144Pr(III) by an intramolecular electron-transfer. The mechanisms and the rate constants are established for the decomposition of the intermediate leading to the formation of the uncomplexed ion. It was also suggested that the uncomplexed 144Pr(III) ion is produced directly by an exhaustive bond-rupture of the daughter complex ion, without any formation of the intermediate. The ratio of bond-rupture was determined to be 0.25; this value is in accordance..." @default.
- W2032982373 created "2016-06-24" @default.
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- W2032982373 date "1969-03-01" @default.
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- W2032982373 title "Chemical Effects Associated with β-Decay Process. IV. Kinetic Studies of the Chemical Behavior of144Pr Decayed from the144Ce(III)-Diethylenetriaminepentaacetate Complex" @default.
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- W2032982373 doi "https://doi.org/10.1246/bcsj.42.696" @default.
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