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- W2033042421 abstract "Abstract In this paper the perturbation expressions of the g z and g x factors of the 3d 9 ions with 2 A 1g ground state in a tetragonal crystal field are obtained by a molecular orbital approach. Using these formulae the g z and g x factors of the NH 4 X : Cu 2+ (X = Cl,Br,I) crystals are calculated. The results show that the contribution of the spin-orbit coupling from ligands in small for the Cu 2+ Cl − cluster but significant for the Cu 2+ I − cluster. The theoretical difficulties of pure crystal-field model in these compounds, namely the sign of the Δg z ( = g z − g s ) in NH 4 I : Cu 2+ being opposite to the experimental, and the order of the g z ( ζ d ) (NH 4 Cl : Cu 2+ > NH 4 Br : Cu 2+ > NH 4 I : Cu 2+ ) being opposite to the measured one (NH 4 Cl : Cu 2+ 4 Br : Cu 2+ 4 I : Cu 2+ ), are hence removed." @default.
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- W2033042421 date "1997-04-01" @default.
- W2033042421 modified "2023-09-27" @default.
- W2033042421 title "g factor of Cu2+ with 2A1g ground state" @default.
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- W2033042421 doi "https://doi.org/10.1016/s0921-4526(96)01151-9" @default.
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