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- W2033063459 abstract "Abstract The solid-state diffusion model of actinide leaching developed in Part II of this series is applied to leaching of radiogenic daughters of the actinide decay chains. For an untreated natural monazite, the direct leaching component of 228Th release is larger than that for 232Th because of enhanced solid-state mobility for 228Th provided by 228Ra-recoil tracks. A significant portion of the 228Th which appears in the leachate, however, is attributed to decay of insoluble 228Ra which is continually released from the mineral by matrix dissolution and recoil ejection. For a monazite sample that was annealed at 800°C prior to leaching, the bulk of the 228Th in solution was supplied by decay of 228Ra rejected from the mineral matrix during annealing. The radiogenic 234U daughter of the 238U decay chain did not exhibit similarly enhanced leaching because the long half-life of 234U permitted local radiation damage to be annealed out at ambient temperature prior to 234U decay." @default.
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- W2033063459 date "1990-07-01" @default.
- W2033063459 modified "2023-10-17" @default.
- W2033063459 title "Leaching of uranium and thorium from monazite: III. Leaching of radiogenic daughters" @default.
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- W2033063459 doi "https://doi.org/10.1016/0016-7037(90)90259-n" @default.
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