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• W2033096733 abstract "We investigated the freezing of colloidal spheres in two dimensions with single-particle resolution. Using micron-size, charge-stabilized polystyrene spheres with a temperature-dependent depletion attraction induced by surfactant micelles, we supercooled an initially amorphous (gaslike) system. Particle motions were monitored as crystallization proceeded. At low concentrations, freezing occurred in a single step in a manner consistent with classical nucleation theory. In other samples two-step nucleation was found, in which amorphous clusters grew to approximately 30 particles, then rapidly crystallized. Measured free energies show the role of metastable gas-liquid coexistence, which also enhanced the rate of nucleation following deeper quenches." @default.
• W2033096733 created "2016-06-24" @default.
• W2033096733 creator A5052721481 @default.
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• W2033096733 date "2009-05-15" @default.
• W2033096733 modified "2023-10-16" @default.
• W2033096733 title "Experimental Evidence for Two-Step Nucleation in Colloidal Crystallization" @default.
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• W2033096733 doi "https://doi.org/10.1103/physrevlett.102.198302" @default.
• W2033096733 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19519003" @default.
• W2033096733 hasPublicationYear "2009" @default.
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