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- W2033106071 abstract "The design and construction of higher-order structure and function in proteinosome microcompartments enclosed by a cross-linked membrane of amphiphilic bovine serum albumin/poly(N-isopropylacrylamide) (BSA-NH2/PNIPAAm) nanoconjugates is described. Three structure/function relationships are investigated: (i) differential chemical cross-linking for the control of membrane disassembly and regulated release of encapsulated genetic polymers; (ii) enzyme-mediated hydrogel structuring of the internal microenvironment to increase mechanical robustness and generate a molecularly crowded reaction environment; and (iii) self-production of a membrane-enclosing outer hydrogel wall for generating protease-resistant forms of the protein-polymer protocells. Our results highlight the potential of integrating aspects of supramolecular and polymer chemistry into the design and construction of novel bioinspired microcompartments as a step toward small-scale materials systems based on synthetic cellularity." @default.
- W2033106071 created "2016-06-24" @default.
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- W2033106071 date "2014-06-16" @default.
- W2033106071 modified "2023-09-29" @default.
- W2033106071 title "Design and Construction of Higher-Order Structure and Function in Proteinosome-Based Protocells" @default.
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- W2033106071 doi "https://doi.org/10.1021/ja504213m" @default.
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