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- W2033428927 abstract "ABSTRACT Previously, we developed a simple, one-parameter model reproducing the observed inhibiting effect of nitrogen species in the hydrodesulfurization (HDS) of hindered sulfur heterocycles. The model owes its simplicity to some nontrivial assumptions. Here we develop a full model by relaxing these assumptions, which gives a more quantitative picture of how sulfur, nitrogen, and catalyst surface interact on many widely disparate time scales. Computational results build a strong case for the accuracy of the previous one-parameter theory. As such, the theory should be applicable to reaction systems in which catalyst poisoning is driven by nonequilibrium adsorption. Some of the complexities and subtleties in modeling the competitive adsorption effects in distillate HDS are discussed, giving special attention to the design of robust catalyst-deactivation-compensation operating strategies." @default.
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- W2033428927 date "2006-04-01" @default.
- W2033428927 modified "2023-10-15" @default.
- W2033428927 title "MODELING OF COMPETITIVE ADSORPTION OF NITROGEN SPECIES IN HYDRODESULFURIZATION" @default.
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- W2033428927 doi "https://doi.org/10.1080/00986440500191669" @default.
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