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• W2033526410 abstract "A sodium cluster ion, Na9+, having a closed electronic shell was allowed to collide with a rare-gas atom (He or Ne), and collisionally fragmented ions were measured by using a tandem mass-spectrometer equipped with several octapole ion guides. The mass spectrum of the product ions show that sodium atom and dimer are released dominantly from the cluster ion, Na9+. The dependencies of the absolute cross sections for the Na and the Na2 release on the collision energy were determined for collision energies up to 3 eV in the center of mass frame. The cross section for the Na2 release increases much more rapidly than that for the Na release as the collision energy increases, while the cross sections for the Na and the Na2 release start to rise at almost the same collision energy of 0.75 ± 0.1 eV. The collision-energy dependencies are explained by orbital correlation diagrams for the Na8+ + Na and the Na7+ + Na2 systems on the basis of a model that a spherical jellium of Na9+ is deformed by collision of a rare-gas atom. The total absolute cross sections are estimated by a two-step scheme: collisional excitation and dissociation." @default.
• W2033526410 created "2016-06-24" @default.
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• W2033526410 date "1996-04-15" @default.
• W2033526410 modified "2023-10-01" @default.
• W2033526410 title "Role of electron pairing in collisional dissociation of Na⁺₉ by a rare‐gas atom" @default.
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• W2033526410 doi "https://doi.org/10.1063/1.471318" @default.
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