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W2033645650 abstract "This paper applies the general methods developed in the previous paper (Paper I) to the case of one-photon, dipole transitions of a molecular solute. The results generalize transient-grating spectroscopy to an arbitrarily number of dimensions. Transition and detection operators are derived, and their matrix elements are calculated in the complex-valued basis set developed in Paper I. Selection rules make it possible to analyze which incoherent pathways, and thus which correlation functions, contribute to an N-dimensional multiple population-period transient spectroscopy experiment. Irreducible-tensor methods allow the amplitudes of the contributing orientational-correlation functions to be calculated for arbitrary polarization conditions. A second-rank polarization tensor is used to describe the polarization of the pair of beams creating or detecting a grating. Several known results for one-dimensional experiments are rederived in this formalism to provide examples of its use." @default.
W2033645650 created "2016-06-24" @default.
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W2033645650 date "2010-04-08" @default.
W2033645650 modified "2023-10-13" @default.
W2033645650 title "Hilbert-space treatment of incoherent, time-resolved spectroscopy. II. Pathway description of optical multiple population-period transient spectroscopy" @default.
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W2033645650 doi "https://doi.org/10.1063/1.3327781" @default.
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