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• W2033648858 abstract "Nanocrystalline diphenylcyclopropenone (DPCP) undergoes a photodecarbonylation reaction to form diphenylacetylene (DPA) with a quantum yield of ∼3, presumably the result of a quantum chain reaction (QCR). We have performed an ultrafast spectroscopic investigation of this process, and found direct evidence that, following photoexcitation of solid DPCP, DPA product molecules appear in a sequential manner over a ∼30 ps time scale. We also see spectroscopic evidence for an excited state of DPCP that is optically inaccessible from the ground state; this state can be populated via short-range energy transfer from excited DPA product molecules, providing a mechanistic explanation of the sequential re-excitation and decarbonylation of DPCP and constituting a direct observation of a QCR." @default.
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• W2033648858 date "2011-12-16" @default.
• W2033648858 modified "2023-09-26" @default.
• W2033648858 title "Ultrafast Spectroscopic Observation of a Quantum Chain Reaction: The Photodecarbonylation of Nanocrystalline Diphenylcyclopropenone" @default.
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• W2033648858 doi "https://doi.org/10.1021/jz201360w" @default.
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