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• W2033764651 abstract "237Np Mössbauer spectroscopy between 77 and 4.2 K was carried out in connection with neutron diffraction studies between 300 and 2 K on the tetragonal intermetallic NpCu4Al8. The Mössbauer spectra give an isomer shift of + 14.3 mm/s vs. NpAl2 indicating the non-Kramers Np3+(5I4)-ion to be present. Below 45 K the onset of magnetic hyperfine splitting is observed. It develops into a fully resolved Zeeman pattern at 4.2 K with Beff≈330 T. Neutron diffraction finds no evidence for magnetic order over the whole temperature range scanned. All these results can consistently be explained by paramagnetic relaxation phenomena involving a low lying Γt5 doublet closely followed by a Γt4 singlet as the tetragonal crystalline field states of the Np3+ ion." @default.
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• W2033764651 date "1985-06-01" @default.
• W2033764651 modified "2023-09-26" @default.
• W2033764651 title "Observation of paramagnetic relaxation in the NpCu 4 Al 8 intermetallic compound" @default.
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• W2033764651 doi "https://doi.org/10.1016/0304-8853(85)90172-6" @default.
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