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- W2034005562 abstract "A favored interpretation of the $ensuremath{gamma}ensuremath{leftrightarrow}ensuremath{alpha}$ phase transition in cerium postulates the transformation of the localized $4f$ state in $ensuremath{gamma}$-Ce to a weakly correlated itinerant $4f$ band in $ensuremath{alpha}$-Ce. However, results of high-energy neutron inelastic scattering measurements, presented here, show clearly that the magnetic susceptibility response from $ensuremath{alpha}$-Ce follows the ${mathrm{Ce}}^{3+}$ form factor despite the large, 30-fold, increase in its spectral width relative to that in $ensuremath{gamma}$-Ce. This observation provides, for the first time, indisputable evidence for the localized character of the $4f$ state in the $ensuremath{alpha}$ phase. The present findings appear consistent with recent calculations combining dynamical mean-field theory with the local density approximation that indicate a strongly correlated $4f$ state in $ensuremath{alpha}$-Ce. The localized $4f$ state is also fundamental to the Kondo volume collapse theories for the $ensuremath{gamma}ensuremath{leftrightarrow}ensuremath{alpha}$ phase transition in cerium." @default.
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- W2034005562 date "2005-12-15" @default.
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- W2034005562 title "Magnetic Form Factor of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mi>α</mml:mi></mml:math>-Ce: Towards Understanding the Magnetism of Cerium" @default.
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- W2034005562 doi "https://doi.org/10.1103/physrevlett.95.256403" @default.
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