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- W2034111130 abstract "A method to study the rotational dynamics of a molecule interacting with a single short laser pulse or a train of pulses is proposed. The method is based on the observation that for such pulses the time propagator, in the $(t,{t}^{ensuremath{'}})$ formalism, can be expressed as a function of approximate Floquet states given by eigenstates of the one-period time-averaged rotational Hamiltonian multiplied by appropriate Fourier functions for the ${t}^{ensuremath{'}}$ coordinate. Each zeroth-order eigenstate can be improved by diagonalizing a small configuration-interaction matrix formed from virtual Hartree-type wave functions. The resulting approximate propagators are more efficient than the usual sudden propagator as they allow one to obtain, in a single step, the propagated wave function at the end of the last pulse of a pulse train." @default.
- W2034111130 created "2016-06-24" @default.
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- W2034111130 date "2004-11-15" @default.
- W2034111130 modified "2023-09-27" @default.
- W2034111130 title "Multiconfigurational pseudo-Hartree approach for the<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:msup><mml:mi>t</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mrow></mml:math>propagator of a molecule in short laser fields" @default.
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- W2034111130 doi "https://doi.org/10.1103/physreva.70.055401" @default.
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