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- W2034117095 abstract "Two diorganotin(IV) complexes, [Me2Sn(4-FC6H4C(O)NHO)2] (1) and [Bu2Sn(4-FC6H4C(O)NHO)2] (2), were synthesized. The action mode of the diorganotin(IV) complexes with adenosine-5′-monophosphate (5′-AMP) or DNA under different conditions and different time was investigated by high-solution 1H NMR and 31P NMR technology and UV spectroscopy. The complexes 1 and 2 which have different carbon chain lengths exhibited different action modes with mononucleotide or DNA. The interaction of 2 with 5′-AMP resulted in significant chemical shift of H(8), H(2) and 31P. A hyperchromic effect of DNA could be observed due to the interaction of 2 with DNA, while interaction of 1 with 5′-AMP or DNA could only cause obvious change of chemical shift of 31P. The results indicate that the complex 2 is the first case which could selectively bind to both the N(1) atom of the base and the phosphate oxygen atom of 5′-AMP near a physiological condition, and may further destroy the helical structure of DNA, while 1 may merely bind to the phosphate oxygen atom of 5′-AMP and cause the contraction of the DNA helical structure. The results first reveal that the organic group R may not only help the membrane transference of the diorganotin compounds but also play an important role in the action mode with DNA." @default.
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- W2034117095 date "2008-04-01" @default.
- W2034117095 modified "2023-10-18" @default.
- W2034117095 title "Interaction of Dialkyltin(IV) Bishydroxamates with 5′-AMP or DNA:the Impact of Carbon Chain Length to Coordination Properties" @default.
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- W2034117095 doi "https://doi.org/10.1002/cjoc.200890118" @default.
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