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- W2034148925 abstract "Charge-transfer reactions of selected ionic redox couples were studied on rotating glassy carbon electrodes covered with conducting polymers of different membrane properties: poly-N-methylpyrrole as the anion exchanger or poly-N-methylpyrrole with immobilized poly(4-styrenesulfonate) ions as the cation exchanging matrix. The electrochemical and spectroscopic (EDAX) results obtained with the redox systems: Fe(CN)3−4−6, Ru(NH3)3+2+, Eu3+/Eu2+, Co(en)3+2+3 and Fe(C2O4)3−4−3 pointed to reactions proceeding at the polymer-solution interface. The data were analysed on the basis of a model in which the charge transfer was regarded as a redox reaction between polymeric sites in the film and the redox species in the solution. The rate of electron transfer was found to be: (i) proportional to the concentration of the oxidized or reduced polymeric sites; (ii) dependent to some extent on the Donnan potential prevailing at the interface; and (iii) correlated with the thermodynamic driving force of the reaction between the polymer and redox species." @default.
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- W2034148925 date "1994-02-01" @default.
- W2034148925 modified "2023-09-24" @default.
- W2034148925 title "Kinetics and mechanism of charge-transfer reactions between conducting polymers and redox ions in electrolytes" @default.
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- W2034148925 doi "https://doi.org/10.1016/0013-4686(94)80057-x" @default.
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