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• W2034155211 startingPage "807" @default.
• W2034155211 abstract "The title reaction (1) was studied at very low total pressures. The activation energy of the chemiluminescent pathway (1a) depends on the wavelength range in which emission is detected. Measurements at 1.27 μ, close to the maximum of the emission spectrum, yield 16.2 kJ mol−1 which presumably equals the activation energy E1a of the chemiluminescence integrated over all wavelengths. The absolute quantum yield at 290 K was determined to be k1a/k1 = 0.20, using the infrared atmospheric band emitted by known concentrations of O2(1Δg) as intensity standard. These results are combined with temperature dependent rate constants of the bulk reaction to yield separate Arrhenius equations, k1a = 2.90 · 10−12 exp(-1951 K/T) cm3 s−1 for the electronically excited product, and k1b = 2.27 · 10−12 exp(-1475 K/T) cm3 s−1 for the dark component of reaction (1). The half-quenching densities of the chemiluminescence were found to be both wavelength- and temperature dependent, following approximately a T0.5 dependence for M = N2." @default.
• W2034155211 created "2016-06-24" @default.
• W2034155211 creator A5016016784 @default.
• W2034155211 creator A5024809735 @default.
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• W2034155211 date "1981-08-01" @default.
• W2034155211 modified "2023-09-26" @default.
• W2034155211 title "Temperature Dependence of the Chemiluminescent Reaction (1), NO + O3 → NO2(2A1; 2B1,2) + O2, and Quenching of the Excited Product" @default.
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• W2034155211 doi "https://doi.org/10.1002/bbpc.19810850814" @default.
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