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• W2034175838 abstract "In this paper, we demonstrate biphasic microfluidic droplets with broadly tunable internal structures, from simple near-equilibrium drop-in-drop morphologies to complex yet uniform non-equilibrium steady-state structures. The droplets contain an aqueous mixture of poly(ethylene glycol) (PEG) and dextran and are dispensed into an immiscible oil in a microfluidic T-junction device. Above a certain well-defined threshold droplet speed, the inner dextran-rich phase is “stirred” within the outer PEG-rich phase. The stirred polymer mixture is observed to exhibit a near continuum of speed and composition-dependent phase morphologies. There is increasing interest in the use of such aqueous two-phase systems in microfluidic devices for biomolecular applications in a variety of contexts. Our work presents a method to go beyond equilibrium phase morphologies in generating microfluidic “multiple” emulsions and at the same time raises the possibility of biochemical experimentation in benign yet complex biomimetic milieus." @default.
• W2034175838 created "2016-06-24" @default.
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• W2034175838 date "2012-04-06" @default.
• W2034175838 modified "2023-09-23" @default.
• W2034175838 title "Tunable spatial heterogeneity in structure and composition within aqueous microfluidic droplets" @default.
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• W2034175838 doi "https://doi.org/10.1063/1.3694841" @default.
• W2034175838 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/3360713" @default.
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