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• W2034183695 endingPage "2722" @default.
• W2034183695 startingPage "2720" @default.
• W2034183695 abstract "Au(25)(SR)(18)(-) belongs to a new type of superatom that features an icosahedral Au(13) core-shell structure and a protective layer of six RS(Au-SR)(2) motifs. This superatom has a magic number of 8 free electrons that fully fill the 1s and 1p levels of the electron-shell model. By applying this superatom concept to the core-substitution chemistry of Au(25)(SR)(18)(-), we first scanned the periodic table for the potential core atom M by applying a simple rule derived from the 8-electron count and then optimized the selected candidates by density functional theory calculations to create many series of M@Au(24)(SR)(18)(q) core-shell nanoclusters. We found that 16 elements from groups 1, 2, and 10-14 of the periodic table can maintain both electronic and geometric structures of the original Au(25)(SR)(18)(-) magic cluster, indicating that the electron-counting rule based on the superatom concept is powerful in predicting viable M@Au(24)(SR)(18)(q) clusters. Our work opens up a promising area for experimental exploration." @default.
• W2034183695 created "2016-06-24" @default.
• W2034183695 creator A5018814519 @default.
• W2034183695 creator A5031199152 @default.
• W2034183695 date "2009-02-23" @default.
• W2034183695 modified "2023-09-23" @default.
• W2034183695 title "From Superatomic Au₂₅(SR)₁₈⁻ to Superatomic M@Au₂₄(SR)₁₈^<i>q</i> Core−Shell Clusters" @default.
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• W2034183695 doi "https://doi.org/10.1021/ic8024588" @default.
• W2034183695 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19236016" @default.
• W2034183695 hasPublicationYear "2009" @default.
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