Matches in SemOpenAlex for { <https://semopenalex.org/work/W2034203566> ?p ?o ?g. }
- W2034203566 abstract "The behavior of molecules confined in a nanoporous material was studied by adsorption from the gas phase with in situ neutron diffraction, with the aid of a high-pressure adsorption apparatus and the General Materials diffractometer (GEM, ISIS). The aim of this work is to establish the combined adsorption/neutron diffraction technique as a unique tool to elucidate both the adsorption mechanism and the structure of molecules confined in nanoporous materials. For this reason, a well-defined mesoporous system (MCM-41) was selected as adsorbent and carbon dioxide as adsorbate, while diffraction measurements have been carried out along a ${text{CO}}_{2}$ adsorption isotherm $(T=253text{ }text{K})$ in the pressure range of 0--18 bar. Small-angle results at low pressures favor the development of an adsorbed film rather than filling of wall microporosity, while diffraction data provide evidence of a distinct molecular arrangement of this adsorbed layer. At higher pressures diffraction data reveal that the structure of the condensed phase is directly comparable to that of bulk liquid ${text{CO}}_{2}$." @default.
- W2034203566 created "2016-06-24" @default.
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- W2034203566 date "2008-09-23" @default.
- W2034203566 modified "2023-09-30" @default.
- W2034203566 title "<i>In situ</i>neutron diffraction study of adsorbed carbon dioxide in a nanoporous material: Monitoring the adsorption mechanism and the structural characteristics of the confined phase" @default.
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- W2034203566 doi "https://doi.org/10.1103/physrevb.78.115424" @default.
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