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- W2034263907 abstract "Abstract Photoinduced electron transfer between [Ru(bpy) 2 mbpy–pyr] 2+ complex, where mbpy = 4-methyl-4′-carbonyl-2,2′-bipyridine and pyr = 1-aminopyrene, and N , N -dimethylaniline (DMA) gives rise to an irreversible process which ultimately leads to the cleavage of the amide bond that links the pyrene to the ruthenium diimine complex. The photochemical reaction under stationary irradiation was monitored by emission and IR spectroscopic techniques as well as by HPLC chromatographic methods. The results suggest that the amide bond fragmentation occurs after the initial electron transfer process, involving the 3 MLCT state of the Ru complex and DMA moiety that results in the formation of [Ru(bpy) 2 mbpy] 2+ complex and pyrene-1-isocyanate primary photoproducts. This last photoproduct suffers hydrolysis in aqueous medium regenerating the 1-aminopyrene ligand and carbon dioxide." @default.
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- W2034263907 date "2005-04-01" @default.
- W2034263907 modified "2023-09-27" @default.
- W2034263907 title "The amide bridge photocleavage in ruthenium bichromophoric complex" @default.
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- W2034263907 doi "https://doi.org/10.1016/j.ica.2005.01.012" @default.
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