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- W2034274286 abstract "Ultraviolet photodissociation of SH (XΠ2, υ″=2–7) and SD (XΠ2, υ″=3–7) has been studied at 288 and 291nm, using the velocity map imaging technique to probe the angular and speed distributions of the S(D21) products. Photodissociation cross sections for the AΣ+2←XΠ2(υ″) and Δ2←XΠ2(υ″) transitions have been obtained by ab initio calculations at the CASSCF-MRSDCI/aug-cc-pV5Z level of theory. Both the experimental and theoretical results show that SH/SD photodissociation from XΠ2 (υ″⩽7) proceeds via the repulsive wall of the AΣ+2 state. The angular distributions of S(D21) indicate that the dissociation approaches the sudden recoil limit of the AΣ+2 state, yielding strongly polarized fragments. The S(D21) atoms are predominantly produced with total electronic angular momentum perpendicular to the recoil axis." @default.
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- W2034274286 date "2007-03-06" @default.
- W2034274286 modified "2023-10-17" @default.
- W2034274286 title "Photodissociation of vibrationally excited SH and SD radicals at 288 and 291nm: The S(D21) channel" @default.
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- W2034274286 doi "https://doi.org/10.1063/1.2646522" @default.
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