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- W2034277646 abstract "Di- and trinuclear complexes of trans-a2PtII (a = NH3 or NH2CH3) and the purine model nucleobases 9-methyladenine (9-MeA), 9-ethyladenine (9-EtA), 9-methylguanine (9-MeGH), and 9-ethylguanine (9-EtGH) have been prepared and characterized. The following five compounds have been studied using X-ray crystallography: trans-[(NH3)2Pt(9-EtA-N7)(9-MeGH-N7)](NO3)2·1.4H2O (1b), trans,trans-{[Cl(NH2CH3)2Pt]2(9-EtA-N1,N7)}(ClO4)2 (2), trans,trans-{[Cla2Pt](N1-9-MeA-N7)Pt(NH3)2(9-MeGH-N7)}(ClO4)3·nH2O (a = NH2CH3, n = 1 (3a); a = NH3, n = 1.8 (3b)), and trans,trans,trans-{[Cl(NH3)2Pt]2(N1-9-MeA-N7)2Pt(NH3)2}(ClO4)4·H2O (5). In all diplatinated adenine species (2, 3a, 3b, and 5) the Pt−N(1) and Pt−N(7) vectors are approximately at right angles, therefore making these complexes potential building blocks for molecular squares, rectangles, and meanders. Two open nucleobase quartets, 4 and 6, consisting of three trans-diamineplatinum(II) entities and four purine nucleobases (two bridging 9-MeA‘s and two terminal 9-MeGH (4) and 9-EtGH (6), respectively) have been isolated and characterized by elemental analysis and 1H and 195Pt NMR spectroscopy." @default.
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- W2034277646 date "1998-06-01" @default.
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- W2034277646 title "Taking Advantage of Right Angles in <i>N1</i>,<i>N7</i>-Diplatinated Purine Nucleobases: Toward Molecular Squares, Rectangles, and Meanders" @default.
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