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• W2034308651 abstract "The depletion of fossil fuels is inevitable and necessitates alternative sources of energy for sustaining life on Earth. In this scenario, the abundant, relatively less expensive copper metal complexes will play a major role. Especially, copper(I) complexes have attracted attention in the past and continue to be an active area of research, mainly because of their diverse structural and photophysical properties. The emissive property of copper(I) complexes is tunable with the help of ligand environments. A traumatic change in luminescence property has been observed when going from homoleptic to heteroleptic copper(I) complexes. The emission intensity and lifetime have been improved using a variety of diphosphine ligands, with wide bite-angles in conjunction with sterically demanding phenanthroline-framework ligands. In addition, it is also very sensitive to the electronic nature of the coordinated ligands. These advancements have been envisaged with the advanced quantum mechanical calculations showing the oxidation of copper(I) to copper(II) species with square planar geometry which eventually becomes nonemissive in nature. Hence, a variety of diphosphines and phenanthroline ligands have been employed to fine tune the emission and lifetime properties. As a result, instead of Ir(III) and Ru(II) complexes, the widely studied and expensive materials, copper(I) complexes have been employed in several applications including photoredox catalysts in various organic reactions. An array of diphosphine and diimine copper(I) complexes, their applications as sensitizers, and photophysical aspects are discussed in this chapter." @default.
• W2034308651 created "2016-06-24" @default.
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• W2034308651 date "1993-07-01" @default.
• W2034308651 modified "2023-10-16" @default.
• W2034308651 title "Structural aspects of red copper(I) compounds" @default.
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• W2034308651 doi "https://doi.org/10.1016/0010-8545(93)85033-z" @default.
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