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- W2034309975 abstract "The 3p Rydberg region of the spectra of acetone and acetone-d6 has been studied by reson-antly enhanced multiphoton ionization and photoacoustic spectroscopies. Differences between the spectra of cold and room temperature samples, between REMPI and PA spectral measure-ments, and between the laser power dependences of the different 3p←X̃ origins have been deduced to arise from a nonadiabatic coupling of the A1 3p Rydberg and A1ππ* states of acetone. The coupling is proposed to arise from a seam of conical intersection between these two A1 states on the CO stretch–C2CO pyramidalization plane. An analogous seam is proposed to exist between the A1 3d Rydberg and A1 ππ* states." @default.
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- W2034309975 date "1997-07-15" @default.
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- W2034309975 title "Nonadiabatic coupling of the 3p Rydberg and ππ* valence states of acetone" @default.
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- W2034309975 doi "https://doi.org/10.1063/1.475152" @default.
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