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• W2034310123 abstract "A series of cobalt complexes bearing N-containing diphosphine PNP ligands has been synthesized and characterized. The nature of the ligand structure affects the binding of the ligand to the cobalt center and determines the coordination geometry of the cobalt complexes. All the complexes have been employed to catalyze the polymerization of 1,3-butadiene, in combination with methylaluminoxane (MAO) or ethylaluminum sesquichloride (EASC) as the cocatalyst. Both the nature of the ligand and the type of cocatalyst had a remarkable influence on the polymerization activity, microstructure and molecular weight of the resulting polymers. The [Co]/MAO catalytic systems resulted in relatively lower conversions of butadiene and cis-1,4 contents in the polymers than the corresponding [Co]/EASC catalytic systems. Upon activation with EASC, the polymerization behaviors of the catalytic systems were also affected by the reaction parameters." @default.
• W2034310123 created "2016-06-24" @default.
• W2034310123 creator A5001937167 @default.
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• W2034310123 date "2012-10-01" @default.
• W2034310123 modified "2023-10-16" @default.
• W2034310123 title "Stereospecific polymerization of 1,3-butadiene catalyzed by cobalt complexes bearing N-containing diphosphine PNP ligands" @default.
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• W2034310123 doi "https://doi.org/10.1016/j.jorganchem.2012.05.051" @default.
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