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- W2034352032 abstract "Polarised picosecond transient grating experiments on azobenzene molecules doping a solution of 4.3 mol of methanol in toluene demonstrate that rotational relaxation is much faster in the bulk fluid than in the fluid embedded in Corning 7930 Vycor glass. As rotational and translational Brownian motions are related to each other, this proves a drastic change in the diffusion coefficients even on a microscopic length scale, which is in contradiction with a previously suggested fractal model. The authors interpret this feature in terms of sticking effects on porous walls. Since macroscopic and microscopic diffusion coefficients can be determined using the same transient grating experiment by looking at the long- and the short-time-scale behaviours, respectively, it is suggested these two techniques are used simultaneously in order to investigate the influence of pore tortuosity and connectivity on the diffusion properties." @default.
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- W2034352032 date "1989-02-06" @default.
- W2034352032 modified "2023-09-26" @default.
- W2034352032 title "Rotational relaxation of azobenzene in porous Vycor glass" @default.
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- W2034352032 doi "https://doi.org/10.1088/0953-8984/1/5/014" @default.
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