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- W2034355744 abstract "Abstract A coherent control scheme is proposed for the orientation of heteronuclear molecules by two-color phase-locked laser excitation. In the case of hexapole state-selected NO, a superposition of both negative and positive ground-state parity levels is formed, where the internuclear axis of the molecule is oriented along the laser polarization axis. The proposed scheme allows rotationally cold distributions of ground-state heteronuclear molecules to be macroscopically oriented, as in the “brute force” dc electric field orientation technique. Computer simulations show that for a typical 1 Σ ground-state diatomic molecule ( B rot = 0.32 cm −1 ) picosecond two-color phase-locked laser excitation can provide orientation during or after the laser pulse." @default.
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- W2034355744 date "1997-06-01" @default.
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- W2034355744 title "Coherent control of molecular orientation" @default.
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- W2034355744 doi "https://doi.org/10.1016/s0009-2614(97)00436-3" @default.
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