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• W2034357797 endingPage "583" @default.
• W2034357797 startingPage "577" @default.
• W2034357797 abstract "Different-shaped one-dimensional (1D) titanic acid nanomaterials (TANs) were prepared by hydrothermal synthesis. By changing the reaction temperature (120, 170 and 200 °C), three kinds of 1D TAN, short-nanotubes (SNT), long-nanotubes (LNT), and nanorods (NR), were obtained. The obtained TANs were characterized by transmission electron microscopy (TEM), high-resolution transmission electron microscopy (HRTEM), powder X-ray diffraction (XRD), and solid-stated diffuse reflectance UV–vis spectra (UV–vis DRS) techniques. Based on these 1D TAN, Eosin Y-sensitized Pt-loaded TAN were prepared by the in situ impregnation and photo-reduction method. Their photocatalytic activity for hydrogen generation was evaluated in triethanolamine (TEOA) aqueous solution under visible light irradiation (λ ≥ 420 nm). The results indicated that the morphology difference led to a significant variation of photocatalytic performance for hydrogen generation, with the activity order as follows: Eosin Y-sensitized Pt-loaded LNT > Eosin Y-sensitized Pt-loaded NR > Eosin Y-sensitized Pt-loaded SNT. The experimental conditions for photocatalytic hydrogen generation such as Pt loading content, the mass ratio of Eosin Y to TAN, and so on, were optimized. As a result, the highest apparent quantum yields of hydrogen generation for Eosin Y-sensitized Pt-loaded SNT, LNT, and NR were 6.65, 17.36, and 15.04%, respectively. The stability of these photocatalysts and the reaction mechanism of the photocatalytic hydrogen generation are also discussed in detail." @default.
• W2034357797 created "2016-06-24" @default.
• W2034357797 creator A5001237699 @default.
• W2034357797 creator A5032455731 @default.
• W2034357797 date "2008-10-01" @default.
• W2034357797 modified "2023-10-17" @default.
• W2034357797 title "Controlled synthesis and photocatalytic investigation of different-shaped one-dimensional titanic acid nanomaterials" @default.
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• W2034357797 doi "https://doi.org/10.1016/j.jpowsour.2008.06.043" @default.
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