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• W2034376948 abstract "In an earlier report we showed that in concentrated carbonate/bicarbonate solutions, simple Cu(II) salts are highly reactive as water oxidation electro-catalysts. We report here, based on earlier results in the literature, that Cu(0) films on a boron-doped diamond substrate are active toward CO2 reduction to CO and formate. The current densities are higher by ∼2.8 fold than a bulk polycrystalline copper electrode due to the enhanced surface area of the electroplated Cu(0) films. When combined, the two half reactions, catalyzed by Cu(II) and Cu(0), provide a basis for the net electrochemical splitting of CO2 into CO/HCOO− and O2 in CO2/HCO3− buffered aqueous solutions. The resulting electrochemical cell is remarkable for the simple nature of the catalysts, solution conditions, and cell configuration." @default.
• W2034376948 created "2016-06-24" @default.
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• W2034376948 date "2013-01-01" @default.
• W2034376948 modified "2023-09-27" @default.
• W2034376948 title "Cu(ii)/Cu(0) electrocatalyzed CO2 and H2O splitting" @default.
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• W2034376948 doi "https://doi.org/10.1039/c3ee24487c" @default.
• W2034376948 hasPublicationYear "2013" @default.
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