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- W2034382476 abstract "MoO3-based materials are known to be appropriate catalysts for the heterogeneous metathesis of light olefins. Classical preparation methods involve the deposition of a Mo oxide phase on the surface of preformed support via impregnation, grafting or thermal spreading. An alternative sol–gel approach for the elaboration of Mo-based catalysts is presented in this article. Mesoporous ternary Si–Al–Mo mixed oxides are prepared in one step, via non-hydrolytic condensation of chloride precursors in non-aqueous media. After calcination, effective catalysts with very good textures and highly dispersed surface molybdenum species are obtained. The Si/Al ratio influences both the texture and the acidity of the materials, which significantly affects the propene self-metathesis activity. The activity also increases with the MoO3 content. The best catalysts with optimized composition significantly outperform the catalysts prepared by other methods." @default.
- W2034382476 created "2016-06-24" @default.
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- W2034382476 date "2012-01-01" @default.
- W2034382476 modified "2023-09-30" @default.
- W2034382476 title "A non-hydrolytic sol–gel route to highly active MoO3–SiO2–Al2O3 metathesis catalysts" @default.
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- W2034382476 doi "https://doi.org/10.1039/c2cy00475e" @default.
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