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- W2034407130 abstract "Spatial pattern formation and wave propagation in surface reactions are often controlled by the chemical diffusion of adsorbed reactant species in mixed adlayers. We characterize the intrinsically coverage-dependent and tensorial nature of such diffusion, emphasizing that these features result from the influence of site-blocking by coadsorbed species, even in the absence of other interactions. The coverage dependence is shown to depend on the relative hop rates of the various reactants. These features are also shown to significantly influence the spatiotemporal behavior in simple, atomistic lattice-gas models of surface reactions. This is illustrated with two examples: trigger wave propagation in a bistable system characteristic of CO oxidation, and the removal of unstable NO+CO adlayers, controlled by dissociation-mediated NO reduction." @default.
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- W2034407130 date "1998-01-01" @default.
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- W2034407130 title "Chemical diffusion in mixed adlayers and wave propagation in surface reactions" @default.
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- W2034407130 doi "https://doi.org/10.1016/s0039-6028(97)00833-9" @default.
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