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- W2034693716 abstract "An analysis of the magnetic behaviour of Cs3V2O2F7 is proposed in terms of isolated binuclear units (V2O2F7)3-. A theoretical approach based on Anderson's model is proposed to describe the exchange interaction between the two V4+ (d1) ions in the binuclear entity. By fitting the experimental magnetic susceptibility, it is shown that the local distortion of the octahedra is very large compared to the exchange parameter and thus using a Heisenberg Hamiltonian appears to be a good approximation. The intracluster exchange is antimagnetic with J/k=13.5 K. This result has been corroborated by specific heat measurements. Good agreement is obtained between experimental data and values calculated using a simple spin-spin coupling and an exchange parameter J/k=13.8 K very close to that obtained from magnetic susceptibility measurements." @default.
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- W2034693716 date "1984-10-01" @default.
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- W2034693716 title "Magnetic and specific heat studies of the (V2O2F7)3- binuclear unit isolated in Cs3V2O2F7" @default.
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- W2034693716 doi "https://doi.org/10.1016/0304-8853(84)90255-5" @default.
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