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- W2034698170 abstract "Nanocrystalline mesoporous TiO2-based catalysts prepared by a surfactant-assisted templating sol–gel process were tested on epoxidation of cyclohexene in tert-butanol–H2O2 system. The mesoporous TiO2 showed exceptional potential for epoxidation of cyclohexene, exhibiting both higher cyclohexene conversion and higher cyclohexene oxide selectivity than non-mesoporous commercial TiO2 powders, i.e. Ishihara ST-01 and Degussa P-25. The oxides of Fe, Co, Ni, and Ru were also loaded by incipient wetness impregnation method onto the synthesized mesoporous TiO2, aiming to enhance the catalytic performance. Among metal oxide-loaded catalysts, RuO2-loaded mesoporous TiO2 was proved to possess noticeably high catalytic performance based on cyclohexene oxide selectivity. The 1 mol% RuO2-loaded mesoporous TiO2 was the best catalyst, showing the highest cyclohexene oxide selectivity and lowest cyclohex-2-en-1-ol (undesired product) selectivity. Plausible reaction pathways were also proposed." @default.
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- W2034698170 date "2005-11-01" @default.
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- W2034698170 title "Catalysis of nanocrystalline mesoporous TiO2 on cyclohexene epoxidation with H2O2: Effects of mesoporosity and metal oxide additives" @default.
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- W2034698170 doi "https://doi.org/10.1016/j.molcata.2005.07.009" @default.
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