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- W2034705186 abstract "We calculate the magnetic susceptibility and g factor of the isolated ${mathrm{C}}_{60}^{mathrm{ensuremath{-}}}$ ion at zero temperature, with a proper treatment of the dynamical Jahn-Teller effect, the associated orbital angular momentum, the Ham-reduced gyromagnetic ratio, and the molecular spin-orbit coupling. A number of surprises emerge. First, the predicted molecular spin-orbit splitting is two orders of magnitude smaller than in the bare carbon atom, due to the large radius of curvature of the molecule. Second, this reduced spin-orbit splitting is comparable to Zeeman energies, for instance, in X-band electron paramagnetic resonance at 3.39 kGauss, and a field dependence of the g factor is predicted. Third, the orbital gyromagnetic factor is strongly reduced by vibron coupling, and so therefore are the effective weak-field g factors of all low-lying states. In particular, the ground-state doublet of ${mathrm{C}}_{60}^{mathrm{ensuremath{-}}}$ is predicted to show a negative g factor of ensuremath{sim}-0.1. textcopyright{} 1996 The American Physical Society." @default.
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- W2034705186 date "1996-12-15" @default.
- W2034705186 modified "2023-10-03" @default.
- W2034705186 title "Surprises in the orbital magnetic moment and<i>g</i>factor of the dynamic Jahn-Teller ion<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msubsup><mml:mrow><mml:mi mathvariant=normal>C</mml:mi></mml:mrow><mml:mrow><mml:mn>60</mml:mn></mml:mrow><mml:mrow><mml:mi mathvariant=normal>−</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:math>" @default.
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- W2034705186 doi "https://doi.org/10.1103/physrevb.54.17184" @default.
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