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• W2034778690 abstract "Six-dimensional quantum calculations of the sticking probability for H2 hitting a Cu(100) surface with off-normal incidence are presented. The multiconfiguration time-dependent Hartree approach is employed for an efficient wave-packet propagation. The sticking probability is calculated for different initial momenta parallel to the surface. In contrast with the picture described in the literature, the sticking probability was found to depend on the parallel momentum. The results are explained by the topology of the potential-energy surface, which shows significant corrugation with a moderate variation of the barrier height with the surface site." @default.
• W2034778690 created "2016-06-24" @default.
• W2034778690 creator A5028033377 @default.
• W2034778690 creator A5058852598 @default.
• W2034778690 date "2005-09-22" @default.
• W2034778690 modified "2023-09-23" @default.
• W2034778690 title "Off-normal incidence dissociative sticking of H2 on Cu(100) studied using six-dimensional quantum calculations" @default.
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• W2034778690 doi "https://doi.org/10.1063/1.2043027" @default.
• W2034778690 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16392510" @default.
• W2034778690 hasPublicationYear "2005" @default.
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