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• W2034792020 startingPage "157" @default.
• W2034792020 abstract "The reaction of NO + H2 on Pt(100) was studied in the 10−6 mbar range between 300 and 800 K with mass spectrometry, work-function measurements, and video LEED. Both multiple steady states and kinetic oscillations were found. The principal reaction products were N2, H2O and NH3, and the activity and selectivity of the reaction were seen to depend on the partial pressure ratio pH2pNo on the surface temperature, and on the degree of surface reconstruction. Whereas the 1 × 1 surface was active for both N2 and NH3 formation, a well-annealed hex phase exhibited a low catalytic activity. The occurrence of defects during the 1 × 1| hex transition was shown to lead to enhanced N2 formation. At low pH2pNo ratios, N2 for while for large pH2pNo ratios, NH3 production was enhanced. Kinetic oscillations, as determined from variations in the and work-function signals, were found between 430 and 445 K." @default.
• W2034792020 created "2016-06-24" @default.
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• W2034792020 date "1992-03-01" @default.
• W2034792020 modified "2023-10-17" @default.
• W2034792020 title "The NO + H2 reaction on Pt(100): steady state and oscillatory kinetics" @default.
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• W2034792020 doi "https://doi.org/10.1016/0039-6028(92)90174-5" @default.
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