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• W2034797811 endingPage "2081" @default.
• W2034797811 startingPage "2077" @default.
• W2034797811 abstract "The polyol synthesis is a popular method of preparing metal nanostructures, yet the mechanism by which metal ions are reduced is poorly understood. Using a spectrophotometric method, we show, for the first time, that heating ethylene glycol (EG) in air results in its oxidation to glycolaldehyde (GA), a reductant capable of reducing most noble metal ions. The dependence of reducing power on temperature for EG can be explained by this temperature-dependent oxidation, and the factors influencing GA production can have a profound impact on the nucleation and growth kinetics. These new findings provide critical insight into how the polyol synthesis can be used to generate metal nanostructures with well-controlled shapes. For example, with the primary reductant identified, it becomes possible to evaluate and understand its explicit role in generating nanostructures of a specific shape to the exclusion of others." @default.
• W2034797811 created "2016-06-24" @default.
• W2034797811 creator A5007242004 @default.
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• W2034797811 date "2008-05-29" @default.
• W2034797811 modified "2023-10-12" @default.
• W2034797811 title "On the Polyol Synthesis of Silver Nanostructures: Glycolaldehyde as a Reducing Agent" @default.
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• W2034797811 doi "https://doi.org/10.1021/nl800910d" @default.
• W2034797811 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18507481" @default.
• W2034797811 hasPublicationYear "2008" @default.
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