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• W2034881509 abstract "A gas phase chemi-ionization process is used to detect O atoms produced by photodissociation of O2 and N2O. For the photon energies used here the accessible O atom states are within the ground 3P levels and the metastable 1D and 1S levels. Kinetic energies of the O atom photofragments are determined using an atomic beam time-of-flight technique, and the O atom angular distributions are determined by varying the angle between the direction of the photon beam and the atomic beam flight path. Dissociative transitions within the Schumman–Runge continuum of O2 and the principal vacuum ultraviolet absorption continuum of N2O yield results in agreement with previous predictions. For the dissociation of O2 at wavelengths of 120 and 124 nm, the principal dissociation products are O(3P)+O(1D); and, at these wavelengths, the O atom angular distribution is consistent with previous conclusions that predissociation is important. Using existing theories of photofragment angular distributions, an asymmetry parameter having a value of (−0.61±0.05) is obtained for predissociation in O2 at the 10.0 and 10.3 eV absorption features." @default.
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• W2034881509 date "1976-12-15" @default.
• W2034881509 modified "2023-09-23" @default.
• W2034881509 title "Kinetic energies and angular distributions of oxygen atom photofragments produced by photodissociation of O2 and N2O in the vacuum ultraviolet" @default.
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• W2034881509 doi "https://doi.org/10.1063/1.433071" @default.
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