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- W2034911221 abstract "Tailoring nanoarchitecture of materials offers unprecedented opportunities in utilization of their functional properties. Nanostructures of vanadium oxide, synthesized by electrochemical deposition, are studied as a cathode material for rechargeable Na-ion batteries. Ex situ and in situ synchrotron characterizations revealed the presence of an electrochemically responsive bilayered structure with adjustable intralayer spacing that accommodates intercalation of Na+ ions. Sodium intake induces organization of overall structure with appearance of both long- and short-range order, while deintercalation is accompanied with the loss of long-range order, whereas short-range order is preserved. Nanostructured electrodes achieve theoretical reversible capacity for Na2V2O5 stochiometry of 250 mAh/g. The stability evaluation during charge–discharge cycles at room temperature revealed an efficient 3 V cathode material with superb performance: energy density of ∼760 Wh/kg and power density of 1200 W/kg. These results demonstrate feasibility of development of the ambient temperature Na-ion rechargeable batteries by employment of electrodes with tailored nanoarchitectures." @default.
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- W2034911221 date "2011-12-23" @default.
- W2034911221 modified "2023-10-18" @default.
- W2034911221 title "Nanostructured Bilayered Vanadium Oxide Electrodes for Rechargeable Sodium-Ion Batteries" @default.
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- W2034911221 doi "https://doi.org/10.1021/nn203869a" @default.
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