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- W2034981870 abstract "Third phase formation is a key issue in the extraction of plutonium in high concentrations by trialkyl phosphates. A number of parameters influence this phenomenon, among which the nature of the extractant (the carbon chain length, branching) is the important one. Studies on third phase formation in thorium extraction could provide insights into the phenomenon, given the challenges in making measurements on plutonium systems. However, the extrapolation of the results obtained for thorium extraction to plutonium systems is difficult in many instances. In the present paper, results of the extensive investigations carried out at IGCAR on third phase formation in the extraction of Th(NO3)4 by trialkyl phosphates (TalP) are presented. The effects of various parameters such as extractant concentration, temperature, structure of diluent, equilibrium aqueous phase acidity and extractant structure on third phase formation in the extraction of Th(NO3)4 by trialkyl phosphates are discussed. Empirical equations to predict Limiting Organic Concentration (LOC) with respect to various parameters for third phase formation in the extraction of Th(NO3)4 by trialkyl phosphates from nitric acid media are also derived and the calculated LOC values are compared with the experimental values. An effort is made to discuss Pu extraction systems based on the bank of data accumulated." @default.
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- W2034981870 date "2010-03-01" @default.
- W2034981870 modified "2023-10-17" @default.
- W2034981870 title "Third phase formation in the extraction of thorium nitrate by trialkyl phosphates" @default.
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- W2034981870 doi "https://doi.org/10.1088/1757-899x/9/1/012056" @default.
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