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• W2035124503 abstract "α-Tocopherol (α-TOH) can be electrochemically oxidized in CH3CN containing Bu4NPF6 in a chemically reversible two-electron/one-proton (ECE) process to form the phenoxonium cation (α-TO+) that is stable for at least several hours at 243 K. In the presence of up to ∼1% CF3SO3H, α-TO+ exists in equilibrium with the α-tocopherol cation radical (α-TOH+•), whereas at concentrations between ∼1−3% CF3SO3H the electrochemical oxidation of α-TOH occurs by close to one-electron to form α-TOH+•. α-TOH+• can be further oxidized in a one-electron process to form the α-tocopherol dication (α-TOH2+). The identity and stability of the phenolic cationic compounds were determined by a combination of electrochemical (cyclic voltammetry and controlled potential electrolysis) and in situ spectroscopic (UV−vis−NIR, FTIR, EPR, and NMR) analysis." @default.
• W2035124503 created "2016-06-24" @default.
• W2035124503 creator A5020466328 @default.
• W2035124503 creator A5055505410 @default.
• W2035124503 date "2004-09-11" @default.
• W2035124503 modified "2023-09-29" @default.
• W2035124503 title "Electrochemically Controlled Chemically Reversible Transformation of α-Tocopherol (Vitamin E) into Its Phenoxonium Cation" @default.
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• W2035124503 doi "https://doi.org/10.1021/ja046648j" @default.
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