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- W2035247966 abstract "The role of surface sites on γ-alumina in the mechanism of hydrolysis of carbonyl sulfide was investigated using a combination infrared cell-recycle flow reactor. Zero-order and first-order behavior were observed for H2O and COS, respectively. The use of acidic (acetic acid) and basic (NaOH, NH3, and pyridine) site-blocking agents reveal basic sites to be essential for the hydrolysis surface reaction. Competitive adsorption of COS and H2O base centers was evident; however, an Eley-Rideal surface reaction mechanism involving adsorbed H2O seemed most compatible with the experimental observations. Catalytic deactivation with time and with exposure to oxygen were evaluated and explanations put forward." @default.
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- W2035247966 date "1984-02-01" @default.
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- W2035247966 title "A study of the kinetics and mechanism of COS hydrolysis over alumina" @default.
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- W2035247966 doi "https://doi.org/10.1016/0021-9517(84)90223-9" @default.
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