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• W2035353290 endingPage "17075" @default.
• W2035353290 startingPage "17070" @default.
• W2035353290 abstract "In this paper, the regulating role of CoOx on deleterious Cl− over PdO/SiO2 for CO oxidation has been thoroughly studied. By comparing the catalyst prepared from Pd(NO3)2 and PdCl2, the deleterious effect of Cl− has been confirmed. The addition of CoOx leads to the significant temperature-dependent variation of catalysts performance. Calcination below 500 °C weakens the interaction between PdCl42- and silica and results in the remarkable agglomeration of Pd on the silica surface and low activity. However, the presence of CoOx is able to inhibit the agglomeration of PdO at high temperature, and leads catalyst showing higher activity. HRTEM and TPR results support this conclusion and indicate a stronger interaction between PdO and CoO in catalyst after the sample calcined at temperature higher than 500 °C, partially because of the complete decomposition of PdCl2 species. The addition of CoOx can stabilize PdO species, which provide more active centers for the adsorption of reactants. Results also indicated that the CO reaction oxidation occurs at the interface between PdO and CoOx." @default.
• W2035353290 created "2016-06-24" @default.
• W2035353290 creator A5001237699 @default.
• W2035353290 creator A5083016057 @default.
• W2035353290 date "2009-09-02" @default.
• W2035353290 modified "2023-10-17" @default.
• W2035353290 title "Regulating Role of Cobalt Oxide on Deleterious Chlorine Ion over PdO/SiO₂ for CO Oxidation" @default.
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• W2035353290 doi "https://doi.org/10.1021/jp904411y" @default.
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