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- W2035612085 abstract "A series of V2O5- and Co3O4-modified ceria/alumina supports and their corresponding gold catalysts were synthesized and their catalytic activities evaluated in the CO oxidation reaction. V2O5-doped solids demonstrated a poor capacity to abate CO, even lower than that of the original ceria/alumina support, owing to the formation of CeVO4. XRD, Raman spectroscopy, and H2-temperature programmed reduction studies confirmed the presence of this stoichiometric compound, in which cerium was present as Ce3+ and its redox properties were avoided. Co3O4-doped supports showed a high activity in CO oxidation at subambient temperatures. The vanadium oxide-doped gold catalysts were not efficient because of gold particle agglomeration and CeVO4 formation. However, the gold–cobalt oxide–ceria/alumina catalysts demonstrated a high capacity to abate CO at and below room temperature. Total conversion was achieved at −70 °C. The calculated apparent activation energy values revealed a theoretical optimum loading of a half-monolayer." @default.
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- W2035612085 date "2012-03-01" @default.
- W2035612085 modified "2023-10-16" @default.
- W2035612085 title "Influence of Vanadium or Cobalt Oxides on the CO Oxidation Behavior of Au/MOx/CeO2-Al2O3 Systems" @default.
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- W2035612085 doi "https://doi.org/10.1002/cctc.201100373" @default.
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